Coherent Vibrational Dynamics
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Coherent Vibrational Dynamics

Guglielmo Lanzani, Giulio Cerullo, Sandro De Silvestri, Guglielmo Lanzani, Giulio Cerullo, Sandro De Silvestri

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eBook - PDF

Coherent Vibrational Dynamics

Guglielmo Lanzani, Giulio Cerullo, Sandro De Silvestri, Guglielmo Lanzani, Giulio Cerullo, Sandro De Silvestri

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Remarkable developments in the spectroscopy field regarding ultrashort pulse generation have led to the possibility of producing light pulses ranging from 50 to5 fs and frequency tunable from the near infrared to the ultraviolet range. Such pulses enable us to follow the coupling of vibrational motion to the electronic transitions in molecules and

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Information

Publisher
CRC Press
Year
2007
ISBN
9781420017519
Edition
1
Topic
Physical Sciences
Subtopic
Chemistry
Index
Chemistry
34
Coherent
Vibrational
Dynamics
SampleĀ 
Lock-inĀ 
Ampliļ¬erĀ 
PDĀ 
ComputerĀ 
ControlledĀ 
DelayĀ 
LineĀ 
(Ļ„)Ā 
OpticalĀ 
ModulatorĀ 
PumpĀ 
BS1Ā 
BS2Ā 
ProbeĀ 
SHGĀ 
12.3Ā 
M1Ā 
AFĀ 
MCĀ 
PDĀ 
DelayĀ 
LineĀ 
NOPA1Ā 
M2Ā 
NOPA2Ā 
FIGURE
1.20
Scheme
of
the
two-color
pump-probe
system
based
on
NOPAs.
BS,
beam
splitters;
AF,
attenuating
ļ¬lter;
M1,
M2,
metal
mirrors;
MC,
monochromator;
PD,
photode-
tector;
SHG,
second-harmonic
generation
crystal
for
auto-/cross-correlation.
Figure
1.20
shows
the
schematic
of
a
two-color
pump-probe
system
based
on
NOPAs,
providing
sub-20-fs
temporal
resolution
[98,
106]
over
a
broad
spectral
range.
The
laser
source
is
a
CPA
Ti:sapphire.
The
system
is
used
to
pump
two
independent
NOPAs,
each
of
which
can
be
conļ¬gured
to
deliver
ultrashort
pulses
from
the
visible
(500ā€“720
nm)
to
the
near-IR
(900ā€“1500
nm).
The
pump-probe
setup
is
designed
to
accommodate
a
broad
range
of
pump
and
probe
wavelengths,
maintaining
a
very
high
temporal
resolution.
It
is
based
on
a
balanced
Michelson
interferometer:
beam
splitters
BS1
and
BS2
consist
of
120-
Ī¼
m-thick
glass
slides
coated
with
Inconel.
This
coating
guarantees
a
nearly
uniform
40%
reļ¬‚ection

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